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Abstract
Despite the great research and development efforts over the last decades, energy storage has yet to be fully developed to meet real-world energy needs. Lithium-ion batteries, which are widely used in consumer electronics, are able to meet the requirements for short-term applications such as backup power supplies, but their high cost and limited cycle life mean that their power storage potential is presently constrained. There is thus a pressing need to develop high-efficiency, low-cost power storage systems that offer similar energy densities. Supercapacitors, which offer almost twice the energy density of batteries (1 MJ/kg as opposed to 0.9 MJ/kg) yet can charge and discharge at a much higher rate (10–100 times their equivalent battery) are considered a viable alternative. However, supercapacitors have, so far, not attracted the same level of attention as batteries.
In this thesis, a systematic investigation into the electrochemical properties of graphene/MnO2 and graphene/MnO2/polyaniline hybrid materials is carried out. The graphene and polyaniline were both conjugated polymer matrices. A two-step approach was used to synthesise graphene-based electrodes using the Hummer’s method and then the non-covalent conjug
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